Journal of Hebei University (Natural Science Edition) ›› 2016, Vol. 36 ›› Issue (5): 462-467.DOI: 10.3969/j.issn.1000-1565.2016.05.003

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Photoluminescence enhancement effect of CH3NH3PbI3 film

DANG Wei1,LIU Xu1,BAI Jingjing1,ZHAO Jinjin2,ZHANG Lianshui1   

  1. 1.Key Laboratory of Hebei Province Optic-electronic Information Materials, College of PhysicsScience and Technology, Hebei University, Baoding 071002, China; 2.College of Materials Science andEngineering, Shijiazhuang Tiedao University, Shijiazhuang 050043, China
  • Received:2016-04-10 Online:2016-09-25 Published:2016-09-25

Abstract: The photoluminescence enhancement of CH3NH3PbI3 film and its effect on carrier recombination dynamics were studied by using photoluminescence spectroscopy.Experimental results demonstrate that the rate of photoluminescence enhancement is higher when the power density of light soaking increases.And oxygen atmosphere is helpful to photoluminescence enhancement of CH3NH3PbI3 film.The reduction of defect density in the film is the main mechanism responsible for the photoluminescence enhancement.Furthermore,the effect of light soaking on the recombination dynamics of free carriers and shallow trapped carriers was analyzed by microwave absorption dielectric spectroscopy. Densities of free carriers and shallow trapped carriers in CH3NH3PbI3 film show an obvious increase after the light soaking.

Key words: CH3NH3PbI3, photoluminescence enhancement, defect, carrier recombination dynamics

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